Title: Reconstructing tritium exposure using tree rings at Lawrence Berkeley National Laboratory, California.

Authors: Love, Adam H; Hunt, James R; Knezovich, John P

Published In Environ Sci Technol, (2003 Oct 01)

Abstract: Annual tritium exposures were reconstructed using tree cores from Pinus jeffreyi and Eucalyptus globulus near a tritiated water vapor release stack. Both tritium (3H) and carbon-14 (14C) from the wood were measured from milligram samples using accelerator mass spectrometry. Because the annual nature of the eucalyptus tree rings was in doubt, 14C measurements provided growth rates used to estimate the age for 3H determinations. A 30-yr comparison of organically bound tritium (OBT) levels to reported 3H release data is achieved using OBT measurements from three trees nearthe stack. The annual average 3H, determined from atmospheric water vapor monitoring stations, is comparable to the OBT in proximal trees. For situations without adequate historical monitoring data, this measurement-based historical assessment provides the only independent means of assessing exposure as compared to fate and transport models that require prior knowledge of environmental conditions and 3H discharge patterns.

PubMed ID: 14572081

MeSH Terms: Environmental Exposure*; Environmental Monitoring/methods*; Environmental Pollutants/analysis*; Environmental Pollutants/pharmacokinetics; Eucalyptus/growth & development*; Models, Theoretical*; Pinus/chemistry; Pinus/growth & development*; Tritium/analysis*; Tritium/pharmacokinetics; Volatilization