Title: Bottom-Up Synthesized All-Thermal-Catalyst Aerogels for Heat-Regenerative Air Filtration.

Authors: Ji, Xiang; Zhao, Jiayuan; Jung, Sung Mi; Hrdina, Amy I H; Wolf, Martin J; Yang, Xiulin; Vaartstra, Geoffrey; Xie, Helen; Luo, Shao-Xiong Lennon; Lu, Ang-Yu; Welsch, Roy E; Wang, Evelyn N; Li, Lain-Jong; Kong, Jing

Published In Nano Lett, (2021 10 13)

Abstract: Airborne particular matter (PM) pollution is an increasing global issue and alternative sources of filter fibers are now an area of significant focus. Compared with relatively mature hazardous gas treatments, state of the art high-efficiency PM filters still lack thermal decomposition ability for organic PM pollutants, such as soot from coal-fired power plants and waste-combustion incinerators, resulting in frequent replacement, high cost, and second-hand pollution. In this manuscript, we propose a bottom-up synthesis method to make the first all-thermal-catalyst air filter (ATCAF). Self-assembled from ∼50 nm diameter TiO2 fibers, ATCAF could not only capture the combustion-generated PM pollutants with >99.999% efficiency but also catalyze the complete decomposition of the as-captured hydrocarbon pollutants at high temperature. It has the potential of in situ eliminating the PM pollutants from burning of hydrocarbon materials leveraging the burning heat.

PubMed ID: 34543039

MeSH Terms: Air Pollutants*/analysis; Catalysis; Hot Temperature; Power Plants